- 龔江 研究員
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【69 Applied Materials Today】 "Cooking carbon in a solid salt": Synthesis of porous heteroatom-doped carbon foams for enhanced organic pollutant degradation under visible light
作者:Jiang Gong, Jinshui Zhang, Huijuan Lin, Jiayin Yuan*
關(guān)鍵字:Poly(ionic liquid); Nitrogen-doped porous carbon foam; Hierarchical pore; Organic pollutant; Catalytic degradation
論文來源:期刊
具體來源:Applied Materials Today 12 (2018) 168-176
發(fā)表時(shí)間:2018年
Porous heteroatom-doped carbons are desirable for catalytic reactions due to their tunable physicochemical properties, low cost and metal-free nature. Herein, we introduce a facile, general bottom-up strategy, so-called “cooking carbon in a solid salt”, to prepare hierarchically porous heteroatom-doped carbon foams by using poly(ionic liquid) as precursor and a common inorganic salt as structural template. The obtained carbon foams bear hierarchical micro-/meso-/macropores, large specific surface area and rich nitrogen dopant. The combination of these favorable features facilitates the catalytic degradation of aqueous organic pollutants by persulfate under visible light irradiation, in which they prevail over the state-of-the-art metal-/carbon-based catalysts.
關(guān)鍵字:Poly(ionic liquid); Nitrogen-doped porous carbon foam; Hierarchical pore; Organic pollutant; Catalytic degradation
論文來源:期刊
具體來源:Applied Materials Today 12 (2018) 168-176
發(fā)表時(shí)間:2018年
Porous heteroatom-doped carbons are desirable for catalytic reactions due to their tunable physicochemical properties, low cost and metal-free nature. Herein, we introduce a facile, general bottom-up strategy, so-called “cooking carbon in a solid salt”, to prepare hierarchically porous heteroatom-doped carbon foams by using poly(ionic liquid) as precursor and a common inorganic salt as structural template. The obtained carbon foams bear hierarchical micro-/meso-/macropores, large specific surface area and rich nitrogen dopant. The combination of these favorable features facilitates the catalytic degradation of aqueous organic pollutants by persulfate under visible light irradiation, in which they prevail over the state-of-the-art metal-/carbon-based catalysts.