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Linear Viscoelasticity of Filled Polymer Melts

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關鍵詞：

linear wscoelasticity filled polymer melts time-temperature-concentration superposition

資料大小：

217K

所屬學科：

分子表征

來源：

第六屆亞歐研討會上處理和性能增強聚合物會議文集（2013.6.2-6 武漢）

簡介：

Filledpolymersexhibitadiverserangeoftheologyvaryingfromsimpleviscousfluidstohighlyelasticsolidswithincreasingfillervolumefraction,9.Theeffectoffillingontheologyiswell-knownintherangeofsmall9wherethereinforcementcouldbeattributedtohydrodynamiceffectscausedbythesolidinclusionsinthemeltstream.Forhigh9wheredirectparticlecontactsdominatethedeformation,astraightforwardsolutionofhydrodynamicequationsisdifficultandtheoreticalmodelsbasedontherealisticstructuralideasarestillmissingsofar.Thetransitionliquid-liketosolid-likeatthelow-frequency(co)zonehasbeenascribedtotheslowdownofchainrelaxationduetopolymeradsorptiononthesurfaceofparticles,thelong-livedchainbridgesbetweentheparticles,thejammednetworkofinteractingparticlesatlowandintermediate9,orthecolloidalandfrictionalinteractionsaswellasbreakdownoflubricatedindirectcontactsbetweenparticlesat9highenough.Wewillshow,however,theso-calledliquid-likeandsolid-likebehaviorssharethecommonmechanism,intheframeworkofaproposed"twophasemodel"appliedtolineardynamictheologyofpolymermeltsfilledwithawiderangeofnanosizedfillers.Atime-concentrationsuperposition(TCS)principlehasbeenappliedtoweaklyattractingcolloidsuspensionsatcontroversyforabout30years.Faitel,sonandYakobsoncl]CreatedTCSprincipleindynamictheologyofliquid-likechalkdispersionsusingamodulusshiftfactoraGdefinedas"strainamplificationfactor".ApplicabilityofthisTCSprinciplec2-4]suggeststhatthefillerphasedoesnotintroduceanychangesindynamicsofthedispersant,atleastat9belowapercolationthreshold體inthehigh-cozone.However,thisTCSprinciplebreaksdowninthelow-cozonewherethecontributionfromtheparticlenetworkseemsdominative.TrappeandWeitzc5]demonstratedanotherTCSprincipleindynamictheologyofsolid-likeCBdispersions(φ>φc。),byintroducingtwoindependentscalingfactorsforbothmodulusandfrequency,aGandam,whichisfurthervalidatedinseveraldispersionsandpolymercomposites[6-13].MoleculardynamicsimulationonanidealizednanofilledelastomerrevealstheTCSprincipletoterminalrelaxationonthechainlengthscalecl4]whilethisprinciplebreaksdownatthesegmentallengthscale.

作者：

Q．Zheng

上傳時間：

2013-06-28 13:58:26

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